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Passive convergence-permeable reactive barrier (PC-PRB): An effective configuration to enhance hydraulic

《环境科学与工程前沿(英文)》 2022年 第16卷 第12期 doi: 10.1007/s11783-022-1591-y

摘要:

● A novel PRB configuration based on passive convergent flow effect was proposed.

关键词: Passive convergence-permeable reactive barrier (PC-PRB)     Permeable reactive barrier configuration     Numerical simulation     Hydraulic performance evaluation     Sensitivity analysis    

Numerical modeling and performance evaluation of passive convergence-permeable reactive barrier (PC-PRB

《环境科学与工程前沿(英文)》 2023年 第17卷 第11期 doi: 10.1007/s11783-023-1731-z

摘要:

● A 2D finite-element solute transport model, PRB-Trans, is developed.

关键词: Passive convergence-permeable reactive barrier     Numerical modeling     Hydraulic behavior assessment     Pollutant treatment performance evaluation     Influential factors analysis    

Nitrobenzene contamination of groundwater in a petrochemical industry site

Yongsheng Zhao, Lin Lin, Mei Hong

《环境科学与工程前沿(英文)》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1107-6

摘要:

The contaminant transport distance is predicted using numerical model.

Zero-valent iron can be used to effectively transform nitrobenzene to aniline.

Experiment shows that two-layer PRB systems have a very good treatment effect.

关键词: Nitrobenzene     Benzene     Groundwater     Zero-valent iron     Permeable reactive barrier    

Magnetohydrodynamic slip flow and diffusion of a reactive solute past a permeable flat plate with suction

Krishnendu BHATTACHARYYA, G. C. LAYEK

《化学科学与工程前沿(英文)》 2011年 第5卷 第4期   页码 471-476 doi: 10.1007/s11705-011-1130-z

摘要: The magnetohydrodynamic (MHD) boundary layer slip flow and solute transfer over a porous plate in the presence of a chemical reaction are investigated. The governing equations were transformed into self-similar ordinary differential equations by adopting the similarity transformation technique. Then the numerical solutions are obtained by a shooting technique using the fourth order Runge-Kutta method. The study reveals that due to the increase in the boundary slip, the concentration decreases and the velocity increases. On the other hand, with an increase in the magnetic field and mass suction, both boundary layer thicknesses decreased. As the Schmidt number and the reaction rate parameter increases, the concentration decreases and the mass transfer increases.

关键词: slip flow     MHD boundary layer     reactive solute diffusion     flat plate     suction/injection    

Effect of a less permeable stronger soil layer on the stability of non-homogeneous unsaturated slopes

Nabarun DEY, Aniruddha SENGUPTA

《结构与土木工程前沿(英文)》 2020年 第14卷 第6期   页码 1462-1475 doi: 10.1007/s11709-020-0674-8

摘要: Slope failure occurs due to an increase in the saturation level and a subsequent decrease in matric suction in unsaturated soil. This paper presents the results of a series of centrifuge experiments and numerical analyses on a 55° inclined unsaturated sandy slope with less permeable, stronger silty sand layer inclusion within it. It is observed that a less permeable, stronger silty sand layer in an otherwise homogeneous sandy soil slope hinders the infiltration of water. The water content of the slope just above the stronger layer increases significantly, compared to elsewhere. No shear band is found to initiate in a homogeneous sandy soil slope, whereas for a non-homogeneous slope, they initiate just above the less pervious, stronger layer. A discontinuity of the shear zone is also observed for the case of a non-homogeneous soil slope. The factor of safety of a non-homogeneous, unsaturated soil slope decreases because of the less permeable, stronger layer. It decreases significantly if this less permeable, stronger soil layer is located near the toe of the slope.

关键词: non-homogeneous slope     stronger soil layer     factor of safety     centrifuge model test     unsaturated soils    

Design and optimization of reactive distillation: a review

《化学科学与工程前沿(英文)》 2022年 第16卷 第6期   页码 799-818 doi: 10.1007/s11705-021-2128-9

摘要: Reactive distillation process, a representative process intensification technology, has been widely applied in the chemical industry. However, due to the strong interaction between reaction and separation, the extension of reactive distillation technology is restricted by the difficulties in process analysis and design. To overcome this problem, the design and optimization of reactive distillation have been widely studied and illustrated for plenty of reactive mixtures over the past three decades. These design and optimization methods of the reactive distillation process are classified into three categories: graphical, optimization-based, and evolutionary/heuristic methods. The primary objective of this article is to provide an up-to-date review of the existing design and optimization methods. Desired and output information, advantages and limitations of each method are stated, the modification and development for original methodologies are also reviewed. Perspectives on future research on the design and optimization of reactive distillation method are proposed for further research.

关键词: reactive distillation     process intensification     design method     reactive phase diagram     optimization algorithm    

Moisture diffusion behavior of permeable fiber-reinforced polymer composite

Jianjiang YANG, Qingsheng YANG, Lianhua MA, Wei LIU,

《机械工程前沿(英文)》 2010年 第5卷 第3期   页码 347-352 doi: 10.1007/s11465-010-0093-y

摘要: A unit cell approach is employed to predict the effective moisture diffusion property in fiber-reinforced biopolymer. The permeable fibers distributed in the matrix are taken as inclusion phases in the system. Based on a unit cell model, the calculation method for moisture diffusion coefficients is developed in this paper. Moisture diffusion property and effective diffusion coefficients are numerically investigated under different temperature and volume fractions of fibers. The calculated results agree well with Gueribiz’s solutions. Therefore, it is reliable in predicting moisture diffusion property of composite using the unit cell model. The present result shows that the effective diffusion coefficient of a composite depends on both temperature and volume fraction of fibers. The effective diffusion coefficient of regular hexagon pattern composite is larger than that of square pattern at the same temperature and volume fraction.

关键词: fiber-reinforced biopolymer     effective diffusion coefficient     unit cell     finite element modeling (FEM)    

Hydrogen production from methanol through dielectric barrier discharge

Baowei WANG, Xu ZHANG, Haiying BAI, Yijun Lü, Shuanghui HU

《化学科学与工程前沿(英文)》 2011年 第5卷 第2期   页码 209-214 doi: 10.1007/s11705-010-1018-3

摘要: The hydrogen fuel cell is a promising option as a future energy resource and the production of hydrogen is mainly depended on fossil fuels now. In this paper, methanol reforming to produce H through dielectric-barrier discharge (DBD) plasma reaction was studied. Effects of the power supply parameters, reactor parameters and process conditions on conversion of methanol and distribution of products were investigated. The best reaction conditions were following: input power (45 W), material of inner electrode (stainless steel), discharge gap (3.40 mm), length of reaction zone (90.00 mm), dielectric thickness (1.25 mm), and methanol content (37.65%). The highest conversion of methanol and the yield of H were 82.38% and 27.43%, respectively.

关键词: methanol     dielectric-barrier discharge     hydrogen     plasma    

Degradation of metronidazole by dielectric barrier discharge in an aqueous solution

Zhipeng Yang, Anxing Lai, Hangyu Chen, Youxiang Yan, Ye Yang, Weiwei Zhang, Lei Wang

《环境科学与工程前沿(英文)》 2019年 第13卷 第3期 doi: 10.1007/s11783-019-1117-4

摘要:

The discharge characteristics during the degradation of MNZ by DBD were investigated.

Increasing the discharge frequency can promote the degradation of MNZ.

MNZ removal reaches 99.1% at the initial concentration of 40 ppm within 120 min.

Coexisting organic matter inhibits the degradation of MNZ.

The energy efficiency of DBD for MNZ removal is higher than other technologies.

关键词: Dielectric barrier discharge     Antibiotic     Metronidazole     Water treatment    

Dielectric barrier micro-plasma reactor with segmented outer electrode for decomposition of pure CO

Baowei Wang, Xiaoxi Wang, Bo Zhang

《化学科学与工程前沿(英文)》 2021年 第15卷 第3期   页码 687-697 doi: 10.1007/s11705-020-1974-1

摘要: Four coaxial cylinder dielectric barrier discharge micro-plasma reactors were designed for the non-catalytic decomposition of pure CO into CO and O at low temperature and ambient pressure. The influence of segmented outer electrodes on the electrical characteristics and the reaction performance was investigated. Experimental results indicated that the introduction of segmented outer electrodes can significantly promote the decomposition of CO . Encouragingly, the highest conversion of 13.1% was obtained at an applied voltage of 18 kV, which was a substantial increase of 39.4% compared to the traditional device. Compared with other types of dielectric barrier discharge plasma reactors, the proposed segmented outer electrode micro-plasma reactor can give a higher CO conversion and acceptable energy efficiency. The increase in conversion can be attributed mainly to the enhanced corona discharge caused by the fringe effect at electrode edges, the increase in energy density and the increase in the number of micro-discharges. In addition, detailed electrical characterization was performed to reveal some trends in the electrical behavior of proposed reactors.

关键词: CO2 decomposition     dielectric barrier discharge     segmented outer electrodes     electrical analysis     reactor design    

Numerical simulations of morphological changes in barrier islands induced by storm surges and waves using

Soumendra Nath KUIRY, Yan DING, Sam S Y WANG

《结构与土木工程前沿(英文)》 2014年 第8卷 第1期   页码 57-68 doi: 10.1007/s11709-014-0235-0

摘要: In this paper, an advanced explicit finite volume flow model in two-dimensions is presented for simulating supercritical coastal flows and morphological changes in a tidal/coastal inlet and barrier islands due to storm surges and waves. This flow model is coupled with existing wave-action model and sediment transport model. The resulting integrated coastal process model is capable of simulating flows induced by extreme conditions such as waves, surge tides, river flood flows, etc., and morphological changes induced by rapid coastal currents and waves. This developed supercritical flow model is based on the solution of the conservative form of the nonlinear shallow water equations with the effects of the Coriolis force, uneven bathymetry, wind stress, and wave radiation stresses. The forward Euler scheme is used for the unsteady term; and the convective term is discretized using the Godunov-type shock-capturing scheme along with the HLL Riemann solver on non-uniform rectilinear grids. The accuracy of the developed model is investigated by solving an experimental dam-break test case. Barrier island breaching, overflow and overwash due to severe storm attack are simulated and the predicted morphological changes associated to the events are analyzed to investigate the applicability of the model in a coast where all the physical forces are present.

关键词: coastal inlet     coastal process modeling     supercritical flow     sediment transport     barrier islands    

Ni/MgO catalyst prepared via dielectric-barrier discharge plasma with improved catalytic performance

Yan LI,Zhehao WEI,Yong WANG

《化学科学与工程前沿(英文)》 2014年 第8卷 第2期   页码 133-140 doi: 10.1007/s11705-014-1422-1

摘要: A Ni/MgO catalyst was prepared via novel dielectric-barrier discharge (DBD) plasma decomposition method. The combined characterization of Brunauer-Emmett-Teller measurement, X-ray diffraction, hydrogen temperature-programmed reduction and transmission electron microscopy shows that DBD plasma treatment enhances the support-metal interaction of Ni/MgO catalyst and facilitates the formation of smaller Ni particles. Sphere-like Ni particles form on plasma treated Ni/MgO catalysts. The plasma treated Ni/MgO catalyst shows a significantly improved low temperature activity and good stability for CO reforming of methane to syngas.

关键词: CO2 reforming     methane     dielectric-barrier discharge (DBD)     plasma     Ni/MgO    

A review on application of dielectric barrier discharge plasma technology on the abatement of volatile

Wenjing Lu, Yawar Abbas, Muhammad Farooq Mustafa, Chao Pan, Hongtao Wang

《环境科学与工程前沿(英文)》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1108-5

摘要:

• Applications of non-thermal plasma reactors for reduction of VOCs were reviewed.

• Dielectric barrier discharge (DBD) plasma was considered.

• Effect of process parameters was studied.

• Effect of catalysts and inhibitors were evaluated.

关键词: Non-thermal plasma (NTP)     Dielectric barrier discharge (DBD)     Volatile organic compounds (VOCs)     Abatement     Input power    

Development of oxide based diffusion barrier coatings for CFC components applied in modern furnaces

Kirsten BOBZIN, Lidong ZHAO, Thomas SCHLAEFER, Thomas WARDA

《机械工程前沿(英文)》 2011年 第6卷 第4期   页码 392-396 doi: 10.1007/s11465-011-0241-z

摘要:

Carbon fibre reinforced carbon (CFC) materials show a high potential for usage in furnaces as sample carriers for example, which is due to their excellent thermal stability compared to steel carriers. Only their tendency to react with different metals at high temperatures by C-diffusion is a disadvantage, which can be solved by application of diffusion barriers. In order to enable the utilization of CFC-carriers for e.g. brazing furnaces, within the frame of this study thermally sprayed diffusion barrier coatings were developed. Coatings of mullite and ZrO2-7%βY2O3 (YSZ) were prepared by air plasma spraying (APS). The coatings were investigated in terms of their microstructure and thermal shock behaviour. In order to prove the suitability of the coatings for the application in brazing furnaces, the wettability of the coating surfaces by a Ni-based brazing alloy was investigated. The results showed that both mullite and YSZ could be deposited on CFC substrates with a bond coat of W or SiC. Both coatings exhibited good thermal shock behaviour and an excellent non-wetting behaviour against the used Ni-based braze alloy.

关键词: diffusion barrier coatings     carbon fibre reinforced carbon (CFC)     plasma spraying     microstructure     furnace    

Conversion of methane through dielectric-barrier discharge plasma

WANG Baowei, CAO Xiaolei, YANG Kuanhui, XU Genhui

《化学科学与工程前沿(英文)》 2008年 第2卷 第4期   页码 373-378 doi: 10.1007/s11705-008-0070-8

摘要: Methane coupling to produce C hydrocarbons through a dielectric-barrier discharge (DBD) plasma reaction was studied in four DBD reactors. The effects of high voltage electrode position, different discharge gap, types of inner electrode, volume ratio of hydrogen to methane and air cooling method on the conversion of methane and distribution of products were investigated. Conversion of methane is obviously lower when a high voltage electrode acts as an outer electrode than when it acts as an inner electrode. The lifting of reaction temperature becomes slow due to cooling of outer electrode and the temperature can be controlled in the expected range of 60°C–150°C for ensuring better methane conversion and safe operation. The parameters of reactors have obvious effects on methane conversion, but it only slightly affects distribution of the products. The main products are ethylene, ethane and propane. The selectivity of C hydrocarbons can reach 74.50% when volume ratio of hydrogen to methane is 1.50.

标题 作者 时间 类型 操作

Passive convergence-permeable reactive barrier (PC-PRB): An effective configuration to enhance hydraulic

期刊论文

Numerical modeling and performance evaluation of passive convergence-permeable reactive barrier (PC-PRB

期刊论文

Nitrobenzene contamination of groundwater in a petrochemical industry site

Yongsheng Zhao, Lin Lin, Mei Hong

期刊论文

Magnetohydrodynamic slip flow and diffusion of a reactive solute past a permeable flat plate with suction

Krishnendu BHATTACHARYYA, G. C. LAYEK

期刊论文

Effect of a less permeable stronger soil layer on the stability of non-homogeneous unsaturated slopes

Nabarun DEY, Aniruddha SENGUPTA

期刊论文

Design and optimization of reactive distillation: a review

期刊论文

Moisture diffusion behavior of permeable fiber-reinforced polymer composite

Jianjiang YANG, Qingsheng YANG, Lianhua MA, Wei LIU,

期刊论文

Hydrogen production from methanol through dielectric barrier discharge

Baowei WANG, Xu ZHANG, Haiying BAI, Yijun Lü, Shuanghui HU

期刊论文

Degradation of metronidazole by dielectric barrier discharge in an aqueous solution

Zhipeng Yang, Anxing Lai, Hangyu Chen, Youxiang Yan, Ye Yang, Weiwei Zhang, Lei Wang

期刊论文

Dielectric barrier micro-plasma reactor with segmented outer electrode for decomposition of pure CO

Baowei Wang, Xiaoxi Wang, Bo Zhang

期刊论文

Numerical simulations of morphological changes in barrier islands induced by storm surges and waves using

Soumendra Nath KUIRY, Yan DING, Sam S Y WANG

期刊论文

Ni/MgO catalyst prepared via dielectric-barrier discharge plasma with improved catalytic performance

Yan LI,Zhehao WEI,Yong WANG

期刊论文

A review on application of dielectric barrier discharge plasma technology on the abatement of volatile

Wenjing Lu, Yawar Abbas, Muhammad Farooq Mustafa, Chao Pan, Hongtao Wang

期刊论文

Development of oxide based diffusion barrier coatings for CFC components applied in modern furnaces

Kirsten BOBZIN, Lidong ZHAO, Thomas SCHLAEFER, Thomas WARDA

期刊论文

Conversion of methane through dielectric-barrier discharge plasma

WANG Baowei, CAO Xiaolei, YANG Kuanhui, XU Genhui

期刊论文